I think some of the nice looking sets like E107, E121-80 are practically impossible to complete since many cards in the set are so rare. If you're looking for a nice set that you should be able to complete over time, I think that the Cracker Jack set is probably still the best choice. Other ideas are:
(1) E95
(2) E93
(3) 1921 E253 Oxford Confectionary
(4) 1926-29 Exhibits
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