I think Jack Barry is the toughest card in the set from a condition standpoint- it's always tilted and/or OC, and I strongly suspect it was stripped up incorrectly on the sheet so when cut it was off.
By far, the hardest card in the set for me and for the 5 or 6 friends I had who collected it at the same time was Grover Cleveland Alexander. Some of the commons in the 120's were tougher than they should have been. I didn't find the high numbers in general any tougher than the others and suspect that might have been misinformation that was passed on as fact for years.
Finding a decent album with string intact was by far tougher than completing the set.
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