Agree go for scarcity but I think it also needs to be popular/(in demand).
I think a fun way is to post and ask everyone if you could afford 1-5 cards with a budget up to 50k what would you purchase. If you can get around 20+ responses then take the cards that get the most votes.
Im guessing the list would have cards like-
1933 Goudey Lajoie
T206 Plank
T206 Magie
1916 Ruth Rookie
E98 Wagner (Black Swamp find)
E98 Cobb (Black Swamp find)
1952 Topps Mantle
Etc
Good luck.
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